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Journal Articles

Flexible fuel cycle system for the effective management of plutonium

Fukasawa, Tetsuo*; Hoshino, Kuniyoshi*; Yamashita, Junichi*; Takano, Masahide

Journal of Nuclear Science and Technology, 57(11), p.1215 - 1222, 2020/11

 Times Cited Count:1 Percentile:11.8(Nuclear Science & Technology)

The flexible fuel cycle initiative system (FFCI system) has been developed to reduce spent fuel (SF) amounts, to keep high availability factor for the reprocessing plant and to increase the proliferation resistance for the recovered Pu. The system separates most U from the SF at first, and the residual material called recycle material (RM) which contains Pu, minor actinides, fission products and remaining U will go to Pu(+U) recovery from the RM for Pu utilizing reactor in future. The Pu utilizing reactor is FBR or LWR with MOX fuel. The RM is the buffer material between SF reprocessing and Pu utilizing reactor with compact size and high proliferation resistance, which can suppress the amount of relatively pure Pu. The innovative technologies of FFCI are most U separation and temporary RM storage. They are investigated by the literature survey, fundamental experiments using simulated material and analyses using simulation code. This paper summarizes the feasibility confirmation results of FFCI.

JAEA Reports

Production and setting of fractional elution facility for recovery of useful rare metals from seawater

Seko, Noriaki; Kasai, Noboru; Tamada, Masao; Hasegawa, Shin; Katakai, Akio; Sugo, Takanobu*

JAERI-Tech 2004-076, 78 Pages, 2005/01

JAERI-Tech-2004-076.pdf:17.11MB

In September 1999, we have soaked 200 kg of fibrous amidoxime adsorbents, synthesized by radiation-induced graft polymerization, into seawater to evaluate their performance. Fractional elution facility was set effectively to elute the rare metals on adsorbents in Mutsu-Establishment. This facility consists of two parts of pre-washing and elution. The present report dealt with planning, manufacture and setting of fractional facility. Marine organism and slime on adsorbent cassette (290$$times$$290$$times$$160 mm) were washed out and every 72 cassettes were set in elution unit (1210$$times$$1210$$times$$H1460 mm) with nonwoven materials as a packing to avoid elution loss. In the elution process alkaline and alkaline earth metals were eluted with low concentration hydrochloric acid (0.01M) and rare metals were eluted with high concentration (0.5M) after the packing of elution unit into fractional elution facility.

JAEA Reports

None

Tokizawa, Takayuki

JNC TN6450 99-001, 39 Pages, 1999/01

JNC-TN6450-99-001.pdf:1.85MB

Journal Articles

Preparation of fibrous adsorbents containing amidoxime groups by radiation-induced grafting and application to uranium recovery from sea water

*; Katakai, Akio; Sugo, Takanobu; *

Journal of Applied Polymer Science, 49, p.599 - 607, 1993/00

 Times Cited Count:59 Percentile:89.91(Polymer Science)

no abstracts in English

JAEA Reports

None

*; *; *; *

PNC TJ6557 91-044, 48 Pages, 1990/08

PNC-TJ6557-91-044.pdf:1.92MB

None

Oral presentation

Decontamination of alkali chloride baths containing nuclear materials by precipitation and distillation techniques; Uranyl chloride precipitation test

Ibe, Junya*; Mitani, Mao*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Asanuma, Noriko*; Matsuura, Haruaki*

no journal, , 

Oral presentation

Uranium recovery from the solution originated sludge waste, 1; Selection of some uranium recovery techniques

Takahatake, Yoko; Saito, Madoka*; Iwamoto, Toshihiro; Watanabe, So; Watanabe, Masayuki

no journal, , 

The sludge contained uranium generated production of nuclear fuel has been storage. The sludge is immersed in some kinds of solution. After immersion, uranium is recovered from the solution. Survey of uranium recovery methods was conducted for realization of technical scale facility which is treated sludge solution. Result of comparison on facility scale, amount of second waste, maturity, merit and demerit, several methods which have to be considered were selected.

Oral presentation

Uranium recovery from the solution originated sludge waste, 3; Evaluation of several extractants on cerium (IV) nitrate separation using thermoresponsive polymer

Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*

no journal, , 

The sludge generated production of nuclear fuel contained uranium has been storage. The sludge is immersed in some kinds of solution. After immersion, uranium is recovered from the solution. Cerium extractive tests using thermoresponsive polymer was carried out on two kinds of extractants. C14-BAMA was found to be superior, and we plan to conduct a uranium study on this extractant.

Oral presentation

Uranium recovery from the solution originated sludge waste, 2; Comparison study of uranyl nitrate separation methods by monoamide extractant

Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Watanabe, Masayuki; Naruse, Atsuki*; Tsukahara, Takehiko*

no journal, , 

The sludge contained uranium generated production of nuclear fuel has been storage. The sludge is immersed in some kinds of solution. After immersion, uranium is recovered from the solution. Solvent extraction method, extraction chromatography and gelling extraction method were conducted on uranyl nitrate solution using monoamide extractant to compare on amount of waste and running cost on each methods. The gelling extraction method was superior to other two methods.

Oral presentation

Uranium recovery from leachate of sludges generated from nuclear fuel fabrication process, 4; Evaluation of oxide conversion condition after temperature swing extraction process

Kai, Masao; Iwamoto, Toshihiro; Saito, Madoka*; Takahatake, Yoko; Watanabe, So; Nakamura, Masahiro; Tsukahara, Takehiko*; Itoda, Naokazu*; Naruse, Atsuki*

no journal, , 

The sludges containing uranium are generated in nuclear fuel fabrication process and have been stored in nuclear fuel fabrication facilities. Uranium is suggested to be selectively recovered from the solution in which the sludges are immersed. In this study, the oxide conversion tests were carried out with the gel obtained by the temperature swing extraction tests with cerium. The most effective heating temperature for the oxide conversion of was determined as 1000 degree Celsius. Based on the results of tests with cerium, the oxide conversion tests with uranium gel were also carried out. The gel was heated at 1000, and products were specified according to analysis data.

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